Enhanced radiative emission rate and quantum efficiency in coupled silicon nanocrystal-nanostructured gold emitters.

نویسندگان

  • Julie S Biteen
  • Domenico Pacifici
  • Nathan S Lewis
  • Harry A Atwater
چکیده

We report local-field-enhanced light emission from silicon nanocrystals close to a film of nanoporous gold. We resolve photoluminescence as the gold-Si nanocrystal separation distance is varied between 0 and 20 nm and observe a fourfold luminescence intensity enhancement concomitant with increases in the coupled silicon nanocrystal/nanoporous gold absorbance cross section and radiative decay rate. A detailed analysis of the luminescence data indicated a local-field-enhanced quantum efficiency of 58% for the Si nanocrystals coupled to the nanoporous gold layer.

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عنوان ژورنال:
  • Nano letters

دوره 5 9  شماره 

صفحات  -

تاریخ انتشار 2005